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Transient absorption spectra of (a) (N-DMBI)2 in MeCN, (b) (N-DMBI)2 in toluene, and (c) (Cyc-DMBI)2 in toluene with excitation at 350 nm in the absence of oxygen. (d) Comparison of temporal evolution of the absorption at 654 nm for both dimers in toluene. (e) Spectra for the two monomeric radicals obtained from M06/6-31G(d,p) TD-DFT calculations.
