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. 2023 Aug 24;14(1):110–132. doi: 10.1016/j.apsb.2023.08.024

Table 4.

Summary of ATPS-based biomaterials with simple structures for drug delivery.

ATPS-based biomaterial used for drug delivery Delivered component The ingredient of the ATPSs The advantage of the materials obtained Ref.
(1) Natural macromolecular monomers
(a) Gelatin microgels EGFP PEG (1.9–12.5 kDa) + gelatin (0.03–100 kDa) The EGFP was encapsulated in the gelatin microgels owing to the electrostatic attraction between gelatin and EGFP 22
(b) Gelatin methacrylate microparticles FGF2 PEG (7.3–9.3 kDa) + gelatin The FGF2 was well loaded and exerted good therapeutic effects 100
(c) HES-HEMA microparticles Lysozyme PEG + HES-HEMA Lysozyme-loaded microparticles released in vitro for more than 4 months 101
(d) CMCH microparticles Naproxen and ropivacaine PEG (10 kDa) + CMCH The microparticles delivering drugs can be embedded in the thermosensitive hydrogels to achieve drug delivery for local wound 102
(e) CMCH microparticles Calcium ions, polymerized dopamine PEG (10 kDa) + CMCH Possessing potential for rapid hemostasis 103
(2) Synthetic macromolecular monomers
(a) PEG-CaM-PEG microparticles VEGF, BMP-2 PEG-CaM-PEG + raffinose + Ca2+ Possessing high encapsulation efficiencies and releasing drugs at a predetermined time 104
(b) Macromonomers hydrogel microparticles BSA and lysozyme Norbornene- and thiol-modified four- and eight-armed poly (ethylene glycol) (10 kDa) + DEX (100–200 kDa) Inhalable controlled drugs release system evading alveolar macrophages 105