AutonoMS offers walkaway
automation of ion mobility mass spectrometry
data collection and analysis. (A) AutonoMS integrates software control
layers with the Agilent RapidFire–6560 ion mobility mass spectrometry
system to provide fully automated data acquisition, raw data handling,
data processing, and metabolomic end-to-end analysis, resulting in
tabular metabolite reports and interactive Skyline documents. (B)
The AutonoMS software stack is hosted on a shared drive between the
6560 and RapidFire control computers. Human laboratory users or an
upstream software agent may trigger AutonoMS runs using a tabular
experiment definition file. The AutonoMS workflow control is written
using Prefect14 which coordinates the event-triggered
actions of modules responsible for instrument file compilation, instrument
control (pywinauto15), postacquisition
raw data handling including ion mobility demultiplexing and CCS calibration
(PNNL PreProcessor16 and DEIMoS17), and metabolomic data analysis (Skyline18,19). Additional modules may be written and incorporated into the workflow
to accommodate different instruments or analysis workflows.