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. 2024 May 2;63(19):8739–8749. doi: 10.1021/acs.inorgchem.4c00344

Table 2. CAMY-B3LYP-D3/STO-TZ2P TDDFT Results, Including Wavelengths (λ), Oscillator Strengths (f), MO Compositions, and Symmetries.

E (eV) λ (nm)a f MO compositionb state symmetry
weight (%) from to
Complex C0
1.88 659.2 (a) 0.56 94.6 HOMO LUMO B
      3.5 HOMO–1 LUMO + 1 B
2.26 548.0 (b) 0.03 58.6 HOMO–1 LUMO A
      39.2 HOMO LUMO + 1 A
2.58 481.2 (c) 1.58 58.5 HOMO LUMO + 1 A
      39.2 HOMO–1 LUMO A
2.99 414.6 (d) 1.04 91.7 HOMO–1 LUMO + 1 B
      3.5 HOMO LUMO B
Complex C1
1.64 758.0 (e) 0.89 94.8 HOMO LUMO A
      2.5 HOMO LUMO + 2 A
1.96 632.9 (f) 0.34 84.0 HOMO LUMO + 1 B
      8.9 HOMO–1 LUMO B
      5.1 HOMO–1 LUMO + 2 B
2.35 527.5 (g) 0.34 84.3 HOMO–1 LUMO B
      11.5 HOMO LUMO + 1 B
2.37 523.5 (h) 0.36 74.9 HOMO–1 LUMO + 1 A
      22.0 HOMO LUMO + 2 A
2.71 457.8 (i) 0.76 72.8 HOMO LUMO + 2 A
      22.9 HOMO–1 LUMO + 1 A
3.11 398.4 (j) 0.81 86.7 HOMO–1 LUMO + 2 B
      4.8 HOMO–1 LUMO B
Complex C2
1.48 839.7 (k) 1.24 89.5 HOMO LUMO B
      7.9 HOMO LUMO + 2 B
1.82 679.4 0.01 75.1 HOMO LUMO + 1 A
      13.3 HOMO–1 LUMO A
      5.3 HOMO LUMO + 3 A
2.01 616.5 (l) 0.36 69.3 HOMO–1 LUMO A
      19.6 HOMO LUMO + 1 A
      8.8 HOMO–1 LUMO + 2 A
2.30 539.9 (m) 0.31 43.8 HOMO–1 LUMO + 1 B
      40.4 HOMO LUMO + 2 B
      7.7 HOMO–1 LUMO + 3 B
      5.3 HOMO LUMO B
2.41 514.4 (n) 0.12 50.5 HOMO–1 LUMO + 1 B
      43.8 HOMO LUMO + 2 B
2.63 471.3 (o) 0.25 77.5 HOMO LUMO + 3 A
      9.0 HOMO–1 LUMO A
      7.8 HOMO–1 LUMO + 2 A
2.84 436.2 (p) 0.90 76.0 HOMO–1 LUMO + 2 A
      13.8 HOMO LUMO + 3 A
      6.5 HOMO–1 LUMO A
3.11 398.9 (q) 0.56 86.0 HOMO–1 LUMO + 3 B
      5.1 HOMO LUMO + 2 B
Complex C3
1.59 778.4 (r) 1.04 86.4 HOMO LUMO B
      10.1 HOMO LUMO + 3 B
1.74 714.1 (s) 0.42 88.6 HOMO LUMO + 1 A
      4.6 HOMO LUMO + 4 A
2.05 604.8 (t) 0.59 63.7 HOMO–1 LUMO A
      17.0 HOMO LUMO + 2 A
      12.9 HOMO–1 LUMO + 3 A
2.12 583.8 0.00 79.3 HOMO LUMO + 2 A
      14.7 HOMO–1 LUMO A
2.26 549.2 (u) 0.46 69.5 HOMO–1 LUMO + 1 B
      14.6 HOMO LUMO + 3 B
      7.9 HOMO–1 LUMO + 4 B
2.46 504.9 (v) 0.06 64.1 HOMO LUMO + 3 B
      20.5 HOMO–1 LUMO + 1 B
      6.4 HOMO–1 LUMO + 2 B
      5.7 HOMO LUMO B
2.61 475.2 0.01 90.7 HOMO–1 LUMO + 2 B
      4.0 HOMO LUMO + 3 B
2.72 455.6 0.03 65.6 HOMO LUMO + 4 A
      16.5 HOMO–1 LUMO + 3 A
      11.5 HOMO–1 LUMO A
2.88 430.8 (w) 0.76 65.3 HOMO–1 LUMO + 3 A
      25.0 HOMO LUMO + 4 A
3.17 391.4 (x) 0.50 84.0 HOMO–1 LUMO + 4 B
      4.7 HOMO–1 LUMO + 1 B
      4.3 HOMO LUMO + 3 B
a

The letters in bold in the second column refer to peak labels in Figure 5.

b

The MOs are visually depicted in Figure 6.