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. 2024 Mar 7;11(18):2308535. doi: 10.1002/advs.202308535

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© 2024 The Authors. Advanced Science published by Wiley‐VCH GmbH

This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.

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a) Chemical formula of the HP18. b) Energy levels of HP18, CROs and CROs‐CG. c) Mott–Schottky plots of a. Bulk‐BtzTp, b. Bulk‐BtzTp‐HP18, c. CRO‐BtzTp, d. CRO‐BtzTp‐HP18, e. CRO‐BtzTp‐Cg, f. CRO‐BtzTp‐HP18. d) Mott–Schottky plots of a. Bulk‐TtzTp, b. Bulk‐TtzTp‐HP18, c. CRO‐TtzTp, d. CRO‐TtzTp‐HP18, e. CRO‐TtzTp‐Cg, f. CRO‐TtzTp‐HP18. e,f) LSV curves of ITO/CuI/Bulk‐BtzTp‐HP18/SnO₂/Pt, ITO/CuI/CRO‐BtzTp‐HP18/SnO₂/Pt, ITO/CuI/CRO‐BtzTp‐Cg‐HP18/SnO₂/Pt, ITO/CuI/Bulk‐TtzTp‐HP18/SnO₂/Pt, ITO/CuI/CRO‐TtzTp‐HP18/SnO₂/Pt, and ITO/CuI/CRO‐TtzTp‐Cg‐HP18/SnO₂/Pt. g–j) LSV curves of ITO/CuI/CRO‐BtzTp‐HP18/SnO₂/Pt, ITO/CuI/CRO‐BtzTp‐Cg‐HP18/SnO₂/Pt, ITO/CuI/CRO‐TtzTp‐HP18/SnO₂/Pt, and ITO/CuI/CRO‐TtzTp‐Cg‐HP18/SnO₂/Pt under constant and chopped light. k,l) CA curves of ITO/CuI/CRO‐BtzTp‐HP18/SnO₂/Pt, ITO/CuI/CRO‐BtzTp‐Cg‐HP18/SnO₂/Pt, ITO/CuI/CRO‐TtzTp‐HP18/SnO₂/Pt, and ITO/CuI/CRO‐TtzTp‐Cg‐HP18/SnO₂/Pt. SECM images of m) ITO/CuI/CRO‐BtzTp‐HP18/SnO₂/Pt, n) ITO/CuI/CRO‐BtzTp‐Cg‐HP18/SnO₂/Pt, o) ITO/CuI/CRO‐TtzTp‐HP18/SnO₂/Pt, and p) ITO/CuI/CRO‐TtzTp‐Cg‐HP18/SnO₂/Pt under constant and chopped light.