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. 2024 Nov 19;146(48):33169–33178. doi: 10.1021/jacs.4c12616

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Thermal properties of the polyIL-in-salt systems. (a) Chemical structures of poly(diallyldimethylammonium) bis(fluorosulfonyl)imide (PDADMAFSI) and lithium (fluorosulfonyl)(trifluoromethanesulfonyl)imide (LiFTFSI). (b) Photographs of polymer electrolytes at the polyIL unit/LiFTFSI cation molar ratios of 2:1, 1:2, and 1:8. (c) DSC thermograms for polymer electrolytes with different LiFTFSI concentrations. (d) Relationship between T_g and the mole fraction of Li salt in both mixed anion system and single anion systems with either a FSI (up to 1:2) or a FTFSI anion (up to 1:8). (e) DSC thermograms of mixed anions and single FTFSI anion systems at a molar ratio of 1:8 after 5 days and 2 months.