Table 3.
Set of Experiment | Objective | Experimental Conditions | |
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1 | Evaluate the effect of the H2O2/Fe(II) molar ratio on CYN degradation | H2O2: 75 µM and Fe(II): 22.1 to 375.0 µM; H2O2/Fe(II) molar ratio: 0.2, 0.4, 0.5, 0.6, 0.8, 1.0, 1.6, and 3.4; Initial pH: 5.0; CYN: 0.05 µM and Matrix: Paranoá Lake water. |
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2 | Assess the effect of H2O2 and Fe(II) dosages on CYN degradation | H2O2: 25 to 100 µM and Fe(II): 62.5 to 250.0 µM; Optimum H2O2/Fe(II) molar ratio from set 1; Initial pH: 5.0; CYN: 0.05 µM and Matrix: Paranoá Lake water. |
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3 | Examine the effect of initial CYN concentration on oxidation efficiency | H2O2 and Fe(II) concentrations from set 1; Optimum H2O2/Fe(II) molar ratio from set 1; Initial pH: 5.0; CYN: 0.05, 0.1 and 0.2 µM and Matrix: Paranoá Lake water. |
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4 | Evaluate the effect of initial pH on CYN degradation | H2O2 and Fe(II) concentrations from set 1; Optimum H2O2/Fe(II) molar ratio from set 1; Initial pH values: 3, 4, 5, 7, 9; CYN: 0.05 µM and Matrix: Paranoá Lake water. |
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5 | Examine the effect of humic acid (HA) and algogenic organic (AOM) matter on CYN degradation | 5.1 | H2O2: 25 to 100 µM and Fe(II): 62.5 to 250.0 µM; Optimum H2O2/Fe(II) molar ratio from set 1; Initial pH: 5.0; CYN: 0.05 µM and Matrix: ultrapure water. |
5.2 | H2O2: 25 to 100 µM and Fe(II): 62.5 to 250.0 µM; Optimum H2O2/Fe(II) molar ratio from set 1; Initial pH: 5.0; HA concentration: 5 mg/L; CYN: 0.05 µM and Matrix: ultrapure water. |
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5.3 | H2O2: 25 to 100 µM and Fe(II): 62.5 to 250.0 µM; Optimum H2O2/Fe(II) molar ratio from set 1; Initial pH: 5.0; CYN: 0.05 µM from Raphidiopsis raciborskii crude extract and Matrix: ultrapure water. |
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6 | Compare the degradation of CYN in methanol–free ultrapure water and ultrapure water containing methanol | 6.1 | H2O2: 25 µM and Fe(II): 7.4 to 125.0 µM; H2O2/Fe(II) molar ratio: 0.2, 0.4, 0.5, 0.6, 0.8, 1.0, 1.6, and 3.4; Methanol: 0 and 513.3 µM; Initial pH: 5.0; CYN: 0.05 µM and Matrix: ultrapure water. |
6.2 | H2O2: 10 to 50 µM and Fe(II): 25 to 125 µM; Optimum H2O2/Fe(II) molar ratio from set 6.1; Methanol: 0 and 513.3 µM; Initial pH: 5.0; CYN: 0.05 µM and Matrix: ultrapure water. |