|
|
Concentration (mol m−3) |
|
|
Mean value of (mol m−3) |
|
|
Membrane coefficient based on the Knudsen diffusion model (mol m−2 pa−1 s−1) |
|
|
Membrane coefficient based on the molecular diffusion model (kg m−2 Pa−1 s−1) |
|
|
Membrane permeation coefficient (mol m−2 pa−1 s−1) |
|
|
Diffusion coefficient of CO2 in gas feed stream (m2 s−1) |
|
|
Diffusion coefficient of CO2 in MEA absorbent feed stream (m2 s−1) |
|
|
Channel thickness (m) |
|
|
Equivalent hydraulic diameter of channel (m),
|
|
|
Deviation of experimental results from the theoretical predictions |
|
|
Further absorption flux enhancement |
|
|
Fanning friction factor |
|
|
Dimensionless Henry’s constant |
|
|
Hydraulic dissipate energy (J kg−1),
|
|
|
Absorption flux improvement |
|
|
Power consumption relative index |
|
|
Mass transfer coefficient in the CO2/N2 gas feed stream (m s−1) |
|
|
Mass transfer coefficient in the MEA absorbent feed stream (m s−1) |
|
|
Equilibrium constant |
|
|
Reduced equilibrium constant |
|
|
Overall mass transfer coefficient of membrane (m s−1) |
|
|
Friction loss (J kg−1),
|
|
|
Channel length () |
|
|
Average molecular weight of CO2 and N2 gas mixture () |
|
|
Number of experimental measurements |
|
|
Saturation vapor pressure in the gas feed flow side () |
|
|
Saturation vapor pressure in the liquid absorbent flow side () |
|
|
Volumetric flow rate of the gas feed stream () |
|
|
Volumetric flow rate of the MEA absorbent stream () |
|
|
Gas constant (8.314 ) |
|
|
Reynolds number |
|
|
Precision index of an experimental measurements of absorption flux (mol m−2 s−1) |
|
|
Mean value of (mol m−2 s−1) |
|
|
Dimensionless Schmidt number |
|
|
Enhanced dimensionless Sherwood number |
|
|
Dimensionless Sherwood number for laminar flow |
|
|
Spiral-ring pitch width (m) |
|
|
Ratio of the various promoter widths inserted |
|
|
Absorption flux () |
|
|
Natural log mean CO2 mole fraction in the membrane |
|
|
Axial coordinate along the flow direction () |
| Greek letters |
|
|
|
Mass-transfer enhancement factor |
|
|
Aspect ratio of the channel |
|
|
Thickness of membrane (µm) |
|
|
Membrane porosity |
|
|
Average velocity () |
|
|
Density (),
|
|
|
Concentration polarization coefficients |
| Subscripts |
|
| 1 |
Membrane surface in CO2/N2 gas feed side |
|
|
Liquid phase on membrane surface on MEA feed stream |
|
|
Gas phase on membrane surface on MEA side |
|
a
|
The CO2 /N2 gas feed stream |
|
b
|
The MEA absorbent feed stream |
|
cor
|
Correlated results |
|
promoter
|
Inserting spiral rings as promoters |
|
empty
|
Empty channel |
|
exp
|
Experimental results |
|
|
Gas feed stream |
|
in
|
At the inlet |
|
|
MEA absorbent feed stream |
|
out
|
At the outlet |
|
theo
|
Theoretical predictions |
| Superscripts |
|
|
uni
|
Uniform promoter widths |
|
des
|
Descending promoter widths |