Methylation of RFs by HemK. (a) Matrix-assisted laser
desorption ionization–time of flight MS analysis of a tryptic digest
of RF1 from CA293(hemK+) or
CK783(ΔhemK). A section of the MS spectrum of the
tryptic digest of RF1-FLAG is shown. The predicted m/z
value for each fragment after correction for the isotopes is indicated.
A peak matching the predicted mass of the 229–245 peptide (1657.8
m/z) was present in the sample from
ΔhemK cells, but this peak was apparently shifted by
14 points (to 1671.9 m/z) in the sample from
hemK+ cells. (b)
SDS/PAGE analysis of in vitro-methylated RFs. The
methylation reaction was performed on a 10-fold larger scale than
described in Table 3 and the samples were subjected to SDS/PAGE (12%
polyacrylamide). 3H-labeled protein was then visualized by
autoradiography. In each reaction, 1 μg of 6×His-HemK was used as
enzyme, and the substrate was: lane 1, 5 μg of BSA; lane 2, 10 μg
of BSA; lane 3, 5 μg of RF1-FLAG; lane 4, 10 μg of RF1-FLAG; lane
5, 5 μg of 6×His-RF2; and lane 6, 10 μg of 6×His-RF2. The
positions of the size markers are shown on the left. (c)
One microgram of RF1-FLAG (lane 1) or 6×His-RF2 (lane 2) was analyzed
by SDS/PAGE with the same size markers as in b and
stained by using Coomassie brilliant blue.