FIGURE 8.

Connectivity schemes compatible with the data and used in the global analysis: (A) inhomogeneous model and (B) homogeneous model. Dynamical states are separated into four classes: excited state (red), ground state (blue), photocycle products (green), and two-photon ionization dynamics (black). ESI1, ESI2, and ESI3 refer to the excited-state lifetimes #1, #2, and #3, respectively. pG is the equilibrated ground-state species, and GSI is the ground-state intermediate. Thick solid arrows represent the initial excitation process from the laser pulse and thin solid arrows dynamics represent the “natural” PP population dynamics. The dashed arrows represent the population transfer dynamics that may be enhanced with the dump pulse.