Table 1.
Transient Kinetics analysis of tRNAHis Variants
tRNA | Single Turnover rate of aminoacyl transfer (sec-1) | Apparent K1/2 for tRNA in single turnover (μM)* | Multiple Turnover rate (sec-1) | [32P] AMP burst amplitude, mol AMP/mol active sites | Burst phase rate of [32P] AMP formation (sec-1) | Linear Turnover Number, [14C]- His-tRNAHis subsat. [ATP] (sec-1) | Linear Turnover Number, [32P]-AMP subsat. [ATP] (sec-1) |
---|---|---|---|---|---|---|---|
Wt | 18.8 | 2.5 | 2.01 | No burst | No burst | 2.31 | 1.74 |
G34U | 12.5 | 20 | 0.37 | No burst | No burst | 0.41 | 0.67 |
5’ppp | 0.141 | 12.5 | 0.195 | 0.669 | 0.349 | 0.0969 | 0.0869 |
C73U | 0.020 | 8 | 0.0063 | 0.578 | 7.920 | 0.00610 | 0.0134 |
This value is calculated as one half the concentration of tRNA required to obtain a limiting (highest) rate of aminoacyl transfer, which can be assumed to reflect saturation for tRNA binding. The apparent K1/2 is higher than reported Km for wild type tRNAs in steady state kinetics, as the latter value reflects the effect of two tRNA molecules binding to dimeric enzyme during the catalytic cycle, whereas single turnover experiments reflect one tRNA binding to the dimer in the first turnover. All values represent the mean of two to three independent determinations. The standard deviations on these values were typically 5-15%.