Table 1.
Percentages of radical pairs that have singlet-yield anisotropy Γ > 5%
| J/mT | D/mT | (1,0) | (2,0) | (1,1) | (3,0) | (2,1) | (4,0) | (3,1) | (2,2) |
|---|---|---|---|---|---|---|---|---|---|
| 0 | 0 | 94.9 | 97.5 | 66.8 | 99.4 | 68.3 | 99.2 | 45.4 | 69.3 |
| −0.333 | 0 | 0.0 | 2.5 | 0.1 | 3.8 | 0.7 | 2.3 | 0.3 | 0.2 |
| −0.333 | +1.0 | 8.5 | 45.9 | 6.5 | 15.9 | 6.3 | 20.1 | 3.0 | 4.2 |
| +0.167 | +1.0 | 42.5 | 30.0 | 29.3 | 8.9 | 7.1 | 1.8 | 1.2 | 1.1 |
The value (n,m) signifies n spin-½ nuclei in radical 1 and m in radical 2. Singlet-yields were calculated for 64,000–117,000 radical pairs for each combination of J and D. See text for further details. Although singlet-yield anisotropies were calculated for an ensemble of ∼105 radical pairs, the parameter space for the n + m = 4 case is so large that the coverage is rather sparse; the entries in this table are therefore underestimates of the percentages of pairs that have Γ > 5%.