Table 2.
Kinetic parameters for wild-type and mutant aminotransferases
| Aspa | Phea | |||||
| kcat/KM (M−1 s−1) × 10−1 | kcat (s) | KM (mM) | kcat/KM (M−1 s−1) × 10−2 | kcat (s−1) | KM (mM) | |
| Aspartate Aminotransferases | ||||||
| WT | 910 (13)b | 159 (2)b | 1.75 (0.04)b | 1.19 (0.03)c | n.s.c | n.s.c |
| T109Sc | 86 (7) | 180 (14) | 21 (3) | 3.0 (0.02) | n.s. | n.s. |
| N297Sc | 280 (12) | 95 (1) | 3.5 (0.2) | 1.56 (0.04) | n.s. | n.s. |
| T109S/N297Sc | 120 (4) | 160 (3) | 12.8 (0.7) | 3.3 (0.2) | n.s. | n.s. |
| Trip | 1560 (90) | 13.4 (0.2) | 0.086 (0.006) | 23 (2) | 34 (2) | 15 (2) |
| Grease | 33 (4) | 0.301 (0.004) | 0.092 (0.009) | 19.4 (9) | 3.4 (0.03) | 1.75 (0.07) |
| Hex | 340 (50) | 7.4 (0.3) | 0.22 (0.04) | 370 (20) | 28.9 (0.5) | 0.78 (0.05) |
| Tyrosine Aminotransferases | ||||||
| WTc | 370 | 140 | 3.8 | 9600 | 250 | 0.26 |
| S109Tc | 390 (70) | 61 (4) | 1.4 (0.7) | 2200 (220) | 137 (17) | 0.6 (0.2) |
| S297Nc | 83 (8) | 76 (7) | 9.1 (0.1) | 870 (250) | 65 (20) | 0.6 (0.4) |
| S109T/S297Nc | 130 (24) | 42 (2) | 2.9 (0.4) | 320 (140) | 131 (48) | 2.5 (1.7) |
| retroGrease | 24 (2) | 21.5 (0.9) | 7.9 (0.9) | 400 (30) | 82 (1.4) | 2 (0.2) |
| retroHEX | 120 (11) | 30 (1) | 2.6 (0.3) | 14 (1) | n.s. | n.s. |
(n.s.) No saturation.
a Conditions: 20 μM PLP, 150–200 μM NADH, 25°C. [MDH] = 0.32–2.4 nM for Asp coupled assay. [HO-HxoDH] = 0.3–3.0 μM for Phe coupled assay. Trip AATase, Hex AATase: 0.2 M TAPS at pH 8.4; 0.1 M KCl; 5 or 10 mM αKG for Trip AATase, 4 mM αKG for Hex AATase. retroHex TATase: 20 mM K phosphate at pH 7.5; Ic maintained at 0.1 M with KCl; 1 mg/mL BSA; 15 mM αKG; [L-Asp] varied from 0.5–12 mM. [L-Phe] varied from 2–24 mM. Grease AATase, retroGrease TATase: 0.2 M TAPS at pH 8.0; 0.1 M KCl; 20 mM αKG for Grease AATase, 30 mM αKG for retroGrease TATase. [L-Asp] and [L-Phe] varied from 1–40 mM. Values for Grease AATase and retroGrease TATase are reported as weighted averages from 3–5 experiments.
bFrom Gloss and Kirsch (1995).
c From Luong and Kirsch (2001).
d From Hayashi et al. (1993). Errors were not reported.