Table 2.
Radical Additions to Pyromeconic Acid Pivalate
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---|---|---|---|---|---|
Ent | R1 | 5:6 | Yld, %a | drb | ee, % 5 (6)c |
1 | i-Propyl 5c | 91:9 | 80 | 99:1 | 70 |
2 | c-Pentyl 5d | 93:7 | 74 | 99:1 | 76 (36) |
3 | c-Hexyl 5e | 92:8 | 55 | 99:1 | 70 |
4 | t-Butyl 5f | 90:10 | 76 | 99:1 | 92 |
5d | t-Butyl 5f | 93:7 | 60 | 99:1 | 92 |
6 | (CH3)2C(CH2)3Cl 5g | 92:8 | 45 | 99:1 | 95 (39) |
Isolated yield.
Diastereomer ratio and site selectivity (5:6) were determined by 1H NMR (400 MHz).
Determined by chiral HPLC.
100 mol% 9.