Table 1.
Mutant | L | Ton | Toff | rms | COTon | [O2]50 calc | [O2]50 obs | n calc | n obs |
---|---|---|---|---|---|---|---|---|---|
w/t | 48,000 | 10 | 500 | 0.0027 | 0.2 | 16.6 | 16.2 | 1.54 | 1.47 |
T72V | 5 | 0 | 550 | 0.0051 | 0.2 | 0.2 | 0.3 | 1.43 | 1.55 |
L73M | 650,000 | 11.6 | 550 | 0.0014 | 0.15 | 31.9 | 34.3 | 1.24 | 1.24 |
F97L | 330 | 33 | 47 | 0.0025 | 0.5 | 1.0 | 1.6 | 1.16 | 1.15 |
I114F | 210,000 | 4.8 | 200 | 0.0015 | 0.2 | 26.5 | 34 | 1.22 | 1.08 |
L is the ratio HbT/HbR for deoxyhemoglobin. Ton is the rate of combination of oxygen with T–state hemoglobin, units are μM(dimer) −1seconds−1. Toff units are seconds−1. r.m.s is the square root of the sum of the squares of differences between observed and calculated values of absorbance for all points in an experiment (usually 14000). COTon units as for oxygen. [O2]50 is the concentration of oxygen (μM) required to give half-saturation using the kinetic parameters listed in the allosteric model. n is Hill’s n, a measure of sigmoidicity. For a dimer its limits are 1, no cooperativity, and 2, full cooperativity. Note that due to experimental error, the results of individual experiments given in the text may not agree with the averaged values of the Table.