Table 1.
Entry | Pd source (mol%) | Cs2CO3(eq.) | Conc.(M) | Yield(%)a | ee(%)b |
---|---|---|---|---|---|
1 | Pd2(dba)3CHCl3(5) | 1.0 | 0.02 | 90 | 84 |
2 | Pd2(dba)3CHCl3(5) | 0.7 | 0.02 | 75 | 92 |
3 | Pd2(dba)3CHCl3(2.5) | 1.0 | 0.02 | 89 | 66 |
4 | Pd2(dba)3CHCl3(1.25) | 1.0 | 0.08 | 75 | 85 |
5 | [Pd(C3H5)Cl]2(2) | 1.0 | 0.17 | 88–93 | 87 |
6 | [Pd(C3H5)Cl]2(1.25) | 1.0 | 0.08 | 83 | 92 |
Isolated yield.
Enantioselectivities were determined by chiral HPLC.