Table 3.
Gaussian resolved peak positions and band assignments from absorption, MCD and TD-DFT spectra of L3.
Band | Energy (cm-1) | ε (M-1cm-1) | MCD/Absa | TD-DFT (cm-1) | Assignment |
---|---|---|---|---|---|
5100 | oop OPh CT | ||||
1 | 7499 | - | 11225 | dxz | |
2 | 9483 | 162 | 0.376 | 15078 | dyz |
3 | 10860 | 321 | 0.100 | 15574 | dz2 |
4 | 14576 | 890 | -0.342 | 16035 | dxy |
5 | 16250 | 548 | -0.205 | 22083 | pyr CT |
6 | 22800 | 137 | -0.379 | 23836 | pyr CT |
7 | 25740 | 685 | -0.178 | 26598 | pyr CT |
8 | 27852 | 1764 | -0.058 | 28216 | ip OPh CT |
Normalized ratio of MCD intensity to absorption intensity. This ratio approximates the relative C/D ratios for mull data, where it is not possible to obtain absolute C/D ratios. Sometimes a CT band might have a high C/D ratio when there is significant amount of metal character in the transition.