Table 3.
S1 and S2 vertical excitation energies (nm) for PSB all-trans-6-s-trans retinal in vacuo at various CI/6-31G* levels along with CASSCF and TD-B3LYP results at the B3LYP/6-31G*-optimized geometry
Method | S1 | S2 |
---|---|---|
TD-B3LYP | 501 | 380 |
CASSCF(12/12)a | 553 | 404 |
CASSCF(6/6) | 382 | 334 |
DDCI2+Q(12/12)a | 545 | 416 |
DDCI2+Q(6/6) | 559 | 385 |
DDACPF/2a-2(12/12)a | 527 | 394 |
DDCI3+Q(6/6) | 640 | 474 |
SORCI+Q(6/6) | 626 | 491 |
MRCISD+Q(6/6) | 604 | 458 |
6-root CAS(12/12) results are given for comparison.