Figure 5.
Tyrosyl radical EPR spectra during reaction of the meclofenamate complex of hPGHS-1 with EtOOH. hPGHS-1 (29 μM heme) pre-treated with 2 equivalents of meclofenamate in 100 mM KPi, pH 7.2, 0.1% Tween-20, was reacted on ice with 5 equiv of EtOOH for ~10 s, frozen, and the first EPR spectrum was recorded. For recording subsequent spectra, the sample was thawed and allowed to react at 0 °C for ~10 s before being re-frozen. The arrow indicates the direction of amplitude changes.