Table 2.
Optimization of reaction conditions of sulfenylation of 1g with 1-phenylsulfanyl[1,2,4]triazole 2b.
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entry | solvent | temp, °C | catalyst | eq. of 2b | yield,a % |
1 | CH2Cl2 | rt | 4c | 2.0 | 79 |
2 | Toluene | rt | 4a | 2.0 | 60 |
3 | Toluene | rt | 4b | 2.0 | 65 |
4 | Toluene | rt | 4c | 2.0 | 91 |
6 | Toluene | 0 | 4c | 3.0 | 97 |
5 | PhH/PhMe (3:1) | −10 | 4c | 3.0 | 96 |
Yield of purified product after chromatographic separation.