Table 8.
Addition of organolithium reagents to imine 11 promoted by 12bc
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|---|---|---|---|---|---|
| entry | R2 | solvent | product | yield, %a | erb |
| 1 | n-Bu | toluene | 19 | 82 | 78.5:21.5c |
| 2 | n-Bu | toluene/Et2O (8:1) | 19 | 90 | 83.0:17.0c |
| 3 | n-Bu | i-Pr2O | 19 | 86 | 84.5:15.5c |
| 4 | n-Bu | Et2O | 19 | 90 | 76.5:23.5c |
| 5 | n-Bu | TBME | 19 | 86 | 74.0:26.0c |
| 6 | Phd | toluene | 20 | 82 | 65.0:35.0e |
| 7 | Phf | toluene/Et2O | 20 | 89 | 50.0:50.0e |
| 8 | CH2=CH | toluene | 21 | 95 | 94.5:5.5e |
| 9 | CH2=CH | i-Pr2O | 21 | 75 | 92.0:8.0e |
Yield of chromatographically homogeneous material.
Determined by CSP-HPLC analysis.
R absolute configuration.
Reaction was performed using 2 equiv of PhLi (Aldrich).
Absolute configuration not determined.
Reaction was performed using 2 equiv of prepared PhLi.
