Table 3.
Rate constants (s–1) determined by time-resolved Raman spectroscopy for the formation (or disappearance) of CBS species following photolysis of CBS-CO.
pH | CBS-5c | CBS-CO | Fe(II)-hCBS (calc) | |
---|---|---|---|---|
R266Ma | 7.6 | 1.8(0.3) × 104 | 1.07(0.16) × 104 | 7.4(2.5) × 103 |
8.5 | 2.0(0.3) × 104 | 1.18(0.17) × 104 | 8.2(2.4) × 103 | |
10.5 | 2.4(0.3) × 104 | 1.33(0.12) × 104 | 1.05(0.23) × 104 | |
WTb | 7.6 | 1.8(0.3) × 104 | 1.32(0.16) × 104 | 4.6(1.4) × 103 |
8.6 | 2.2(0.7) × 104 | 1.8(0.4) × 104 | 4.0(2.2) × 103 | |
10.5 | 2.1 (0.3) × 104 | 1.49(0.16) × 104 | 6.4(1.6) × 103 |
This work.
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