TABLE 2.
| |||||
---|---|---|---|---|---|
product | methoda | R | X1 | X2 | yieldb (%) |
5a | I | H | Cl | H | 33 |
5b | I | H | Br | H | 46 |
5c | I | H | I | H | 50 |
6a | II | H | Cl | Cl | 35 |
6b | II | H | Br | Br | 79 |
7a | III | H | NH2 | Cl | 51 |
7b | III | H | NH2 | Br | 94 |
8 | III then I | H | I | Cl | 42 |
9 | III then I | H | Cl | Br | 13 |
11 | I | CN | Br | H | 32 |
See Scheme 2 and the Experimental Section for details
Yields are for isolated pure materials.