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Parameters used for simulation of polarization dependent 2D IR absorptive spectra and linear FTIR spectra of DGdm+ in D2O and 59%D-glycerol/D2O.
| Parameters | Solvent | ||
|---|---|---|---|
| D2O | 59% D-glycerol/D2O | ||
| ω1, cm−1 | 1593.0 | 1588.0 | |
| ω2, cm−1 | 1603.7 | 1602.3 | |
| Δ1, cm−1 | 25 | 18 ± 1 | |
| Δ2, cm−1 | 25 | 11 ± 1 | |
| Δc, cm−1 | 5 ± 1 | 5 ± 1 | |
| D∥, D⊥, *10−10 s−1 | 3.3 | 0.33 | |
| μ1/μ2 | 1 | 0.905 | |
| ket, ps−1 | 0.53 | 0.71 | |
| 〈δωi(τ)δωi(0)〉 | γ, ps−1 | 0.84 | 0.51 |
| Δ, ps−1 | 2.0±0.4 | 1.45±0.15 | |
| τ, ps | 1.13±0.88 | 1.5±0.5 | |
