Dependence of the exchange rate of Hisα103(G10) Nɛ2H
proton on pH (A), and on the concentration of
H+ ions in the pH range from 5.6 to 7.6 (B).
(♦, ⋄) deoxy Hb; (●, ○) HbCO; (▾, ▿) oxy
Hb; (□) CN-met Hb; (▵) azido-met Hb. Filled
symbols: 0.1 M Bis-Tris with 0.18 M chloride ions. Open symbols: 0.1 M
Tris with 0.18 M chloride ions. The solid lines correspond to nonlinear
least-squares fits to Eq. 3 with the following fitted
parameters: kop = (105 ± 16)
s−1,
kOH/kH
= (6.0 ± 1.1) 10−3,
kw/kH
= (1.2 ± 0.4) 10−7 M and
(kop +
kcl)/kH
= (6.2 ± 2.6) 10−7 M for deoxy Hb A, and
kop = (76 ± 5)
s−1,
kOH/kH
= 0,
kw/kH
= (9.4 ± 1.4) 10−8 M and
(kop +
kcl)/kH
= (1.6 ± 0.2) 10−6 M for ligated Hb A.