Table 4.
entry | N-Boc pyrrolidine | R1 | R2 | pyrrolidine | yield (%) | ligand | yield (%) |
---|---|---|---|---|---|---|---|
1 | 10a | C6H5 | H | 12a | 92 | L34 | 38 |
2 | 11ab | C6H5 | 2-OMeC6H4 | 12ab | 97 | L35 | 81 |
3 | 11ac | C6H5 | 2-Naphthyl | 12ac | 100 | L36 | 82 |
4 | 11ba | 2-MeOC6H4 | 2-MeOC6H4 | 12ba | 71 | L37 | 41 |
5 | 11ca | 2-Naphthyl | 2-Naphthyl | 12ca | 98 | L38 | 84 |
6 | 11cb | 2-Naphthyl | 1-Naphthyl | 12cb | 100 | L39 | 77 |
7 | 11cc | 2-Naphthyl | 3,5-t-BuC6H3 | 12cc | 86 | L40 | 68 |
8 | 11d | 3-Biphenyl | 3-Biphenyl | 12d | 97 | L41 | 40 |
9 | 11e | 3,5-PhC6H3 | 3,5-PhC6H3 | 12e | 92 | L42 | 68 |
10 | 11f | 4-Biphenyl | 4-Biphenyl | 12f | 99 | L43 | 82 |
11 | 11g | 1-Naphthyl | 1-Naphthyl | 12g | 10a | L44 | 60 |
Isolated yield for two steps from 10g