Table 5.
Influence of Ring Size of Additive on Enantioinduction.
Entrya | n | Temp. (°C) | Additive | ee (%)b |
---|---|---|---|---|
1 | 1 | rt | 17 | 65 |
2 | 1 | −20 | 17 | 82 |
3 | 1 | −20 | 17 | 95c |
4 | 2 | −20 | 18 | 79 |
5 | 4 | −20 | 19 | 80 |
All reactions run on a 0.47 mmol scale at 1M concentration in both donor and acceptor.
Determined by chiral HPLC.
Diazoester 2 added via slow addition using a syringe pump.