Table 4.
R1 | R2 | 4 (CypA) | 5 (CypA) | 4 (CypB) | 5 (CypB) |
---|---|---|---|---|---|
Cl | Cl | 0.0 | 0.0 | 0.0 | 0.0 |
Cl | F | −0.24 | 0.04 | 0.0 | 0.44 |
F | Cl | 0.33 | 0.17 | 0.68 | 0.74 |
F | F | 0.41 | −0.27 | 0.66 | 0.90 |
Cl | H | 0.80 | −0.79 | 0.89 | 0.20 |
H | Cl | −1.06 | −1.54 | −0.91 | 2.06 |
H | H | −1.68 | −2.02 | 0.52 | 1.76 |
Positive ΔΔGbind value means R1 = R2 = Cl was preferred, and negative means new mutation is preferred. R1 signifies that the substituent is pointing in towards the enzyme and R2 is pointing out towards the aqueous solvent environment.