Table 3.
| |||||
---|---|---|---|---|---|
entrya,b | 3 | R | R' | % yieldb | % eed |
1 | 3a | H | 92 | >99 | |
2 | 3b | Me | 75 | >99 | |
3c | 3c | Me | 62 | 99 | |
4 | 3d | H | 91 | >99 | |
5 | 3e | H | 59 | 99 | |
6c | 3f | H | 75 | >99 | |
7 | 3g | H | 75 | 97 | |
8 | 3h | H | 73 | 99 | |
9c | 3i | H | 73 | 96 | |
10 | 3j | H | 94 | 95 |
Conditions: CDCl3 (0.1 M), 5 mol % A8 · (AuCl)2, 10 mol % AgOTf for 4 h at 0 °C.
Isolated yield of product after column chromatography.
At room temperature.
Determined by chiral HPLC.