Table 3.
Entry | Solvent | Conv. (%)b |
---|---|---|
1 | 5% DMSO-DMF | 81 |
2 | 5% DMSO-DMFc | 85 |
3 | DMSO | 32 |
4 | DMF | 53 |
5 | xylenes | 73 |
6 | MeOHd | 43 |
7 | MeOH | 70 |
8 | EtOH | 56 |
9 | CF3CH2OH | 58 |
10 | i-PrOH | 81 |
Reaction conditions: initial concentration [6] = 0.10 M and [Pd(O2CCF3)2] = 0.020 M, 10 equiv CF3CO2H, 3.0 mL solvent, 70 °C, 24 h.
GC monitoring with biphenyl as internal standard.
Distilled solvents.
No added CF3CO2H.