Table 3.
| ||||
---|---|---|---|---|
Entry | Nucleophile (equiv) | R | Product | Yield (%)a |
1 | Bu4NOAc (1.5) | Ac | 61, 61′ | 74b |
2 | EtOH (56) | Et | 62, 62′ | 56c |
3 | H2O (125) | H | 63, 63′ | 41b |
4 | -- | CH(CF3)2 | 64, 64′ | 33c |
5 | CsOH•H2O (1.5) | H | 63, 63′ | 45b,d |
Isolated as a 1:1 mixture of diastereomers in all cases.
NBS used.
Br(coll)2ClO4 used.
19% of 64, 64′ also isolated.