Truncated molecular orbital diagram of (smif)Ti(dpma) (4; the dpma is in the xz plane, the smif is in the yz plane) illustrating orbitals near the HOMO/LUMO gap. The left side of the diagram features orbitals with dpma character, while the right side pictures those with smif character. The SOMOs whose electrons are AF-coupled to afford the ground state singlet are at ~−2.0 eV; the left orbital is ~50% dxy while the right orbital is ~67% smif Π*, with some dxz admixed. The remaining orbitals with predominantly d-character are not shown, but dxz and dyz are ~ −0.17 and −0.40 eV, respectively, while the σ*-orbitals (dz2 and dx2-y2) are at ~ +1.4 and +2.0 eV.