Nanoimprint lithography was employed to imprint the nanofeatures from nanofeatured molds into polystyrene or polypropylene thin films. Scanning electron microscopy (SEM) images reveal (a) a polystyrene thin film with features having an aspect ratio of 0.88, (b) a polypropylene thin film with features having an aspect ratio of 20, (c) a polystyrene thin film with hierarchical nanofeatures having aspect ratios of 0.5, 1.4, and 3.4, and (d) a polystyrene thin film with features having an aspect ratio of 5.