Table 2.
| ||||||
---|---|---|---|---|---|---|
entry | mol % 10/mol % BzOH | time d | temp °C | solvent | % convn | % ee |
1 | 10/0 | 1 | 23 | CDCl3 | <5 | ND |
2 | 10/5 | 0.4 | 23 | CDCl3 | 90 | 83 |
3 | 10/10 | 0.4 | 23 | CDCl3 | 92 | 80 |
4 | 10/20 | 0.4 | 23 | CDCl3 | 93 | 82 |
5 | 5/5 | 2 | 23 | CDCl3 | 96 | 85 |
6 | 2/2 | 4 | 23 | CDCl3 | 94 | 84 |
7 | 5/5 | 2 | 0 | CDCl3 | 95 | 72 |
8 | 10/5 | 2 | −20 | CDCl3 | 94 | 55 |
9 | 5/5 | 1 | 45 | CDCl3 | 91 | 84 |
10 | 5/5 | 2 | 23 | C6D6 | 98 | 80 |
11 | 5/5 | 2 | 23 | CH2Cl2 | 95 | 74 |
12 | 5/5 | 2 | 23 | CH3CN | 85 | 66 |
13 | 5/5 | 2 | 23 | THF | <5 | ND |
Conversion in all cases was determined by 1H NMR.