Table 3.
Optimization of the asymmetric cyano-TMM cycloaddition using oxindole 46 (R = Moc).
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All reactions were performed at 0.2 M in toluene with 1.5 equivalents 45, 2.5 mol% Pd2(dba)3•CHCl3 and 10 mol% ligand for 12 hours. Yields were combined, isolated product; ee’s were determined by chiral HPLC.
