Table 3.
Scope of the AROCM Reaction with respect to Terminal Olefin[a]
![]() | ||||
---|---|---|---|---|
R2 | Product | Yield [b] | % Z[c] | ee Z[d] (ee E)[d] |
OH |
7e
![]() |
62 | 89 | 93 (86) |
OBz |
7f
![]() |
61 | 88 | 97 (88) |
OTBS |
7g
![]() |
68[e] | 87 | 89 (77) |
OBn |
7h
![]() |
64 | 86 | 91 (nd) |
4-MeOPh |
7i
![]() |
76 | 90 | 93 (79) |
CH2C(O)CH3 |
7j
![]() |
65 | 90 | 92 (84) |
BPin |
7k
![]() |
50 | nd[f] | 91 (nd) |
0.1 mmol cyclobutene, 0.7 mmol terminal olefin.
Combined isolated yield of E and Z products.
Determined by 500 MHz 1H NMR analysis of crude reaction mixture.
Determined by chiral SFC.
Yield determined after derivatization to 7e.
Not determined due to instability of E product.