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(A) The conceptual approach to combine a basic residue and the catalytic biotinylated RhCp*biotinCl2 to achieve a synergistic catalyst. (B) The structure of RhCp*biotinCl2 and the reaction it catalyzes. (C) Proposed transition state for the C–H bond activation. (D) Auto-Dock model showing the spatial relationship of the biotinylated RhCpbiotin(OAc)2 catalyst in the Sav tetramer active site. Reproduced with permission from ref 559. Copyright 2012 AAAS.
