Table 4. Results of a Statistical Analysis Performed by Accounting for Solvent Effects with Various Modelsa.
| method | solvent | MSE | MAE | SD | Max(+) | Max(−) | R2 |
|---|---|---|---|---|---|---|---|
| TD-M06-2X | gas | 0.264 | 0.279 | 0.214 | 0.142 | –0.783 | 0.859 |
| LR,eq | 0.064 | 0.168 | 0.193 | 0.324 | –0.465 | 0.886 | |
| cLR,eq | 0.220 | 0.235 | 0.182 | 0.143 | –0.755 | 0.898 | |
| cLR,neq | 0.221 | 0.236 | 0.183 | 0.143 | –0.758 | 0.897 | |
| cLR,eq (SMD) | 0.209 | 0.225 | 0.177 | 0.143 | –0.728 | 0.904 | |
| CIS(D) | gas | 0.293 | 0.312 | 0.231 | 0.579 | –0.864 | 0.886 |
| LR,eq | 0.094 | 0.176 | 0.196 | 0.380 | –0.545 | 0.926 | |
| cLR,eq | 0.249 | 0.263 | 0.195 | 0.467 | –0.669 | 0.919 | |
| cLR,eq (SMD) | 0.239 | 0.254 | 0.195 | 0.446 | –0.669 | 0.921 | |
| ADC(2) | gas | 0.010 | 0.153 | 0.195 | 0.449 | –0.424 | 0.907 |
| LR,eq | –0.189 | 0.215 | 0.168 | 0.534 | –0.302 | 0.937 | |
| cLR,eq | –0.034 | 0.141 | 0.177 | 0.564 | –0.405 | 0.923 | |
| cLR,eq (SMD) | –0.044 | 0.146 | 0.180 | 0.618 | –0.414 | 0.922 | |
| CC2 | gas | 0.072 | 0.148 | 0.179 | 0.281 | –0.474 | 0.907 |
| LR,eq | –0.128 | 0.163 | 0.147 | 0.489 | –0.288 | 0.940 | |
| cLR,eq | 0.028 | 0.131 | 0.165 | 0.468 | –0.412 | 0.921 | |
| cLR,eq (SMD) | 0.018 | 0.133 | 0.167 | 0.522 | –0.412 | 0.920 | |
| SCS-CC2 | gas | 0.243 | 0.247 | 0.159 | 0.064 | –0.708 | 0.927 |
| LR,eq | 0.044 | 0.110 | 0.133 | 0.254 | –0.384 | 0.952 | |
| cLR,eq | 0.199 | 0.204 | 0.128 | 0.126 | –0.559 | 0.952 | |
| cLR,eq (SMD) | 0.189 | 0.196 | 0.128 | 0.180 | –0.481 | 0.953 | |
| SOS-CC2 | gas | 0.326 | 0.326 | 0.161 | –0.048 | –0.854 | 0.926 |
| LR,eq | 0.129 | 0.158 | 0.148 | 0.198 | –0.683 | 0.940 | |
| cLR,eq | 0.282 | 0.282 | 0.125 | –0.041 | –0.705 | 0.955 | |
| cLR,eq (SMD) | 0.271 | 0.272 | 0.124 | 0.013 | –0.627 | 0.955 | |
| BSE/GW | gas | 0.062 | 0.182 | 0.220 | 0.400 | –0.538 | 0.858 |
| LR,eq | –0.137 | 0.187 | 0.178 | 0.548 | –0.216 | 0.906 | |
| cLR,eq | 0.018 | 0.147 | 0.177 | 0.401 | –0.452 | 0.905 | |
| cLR,eq (SMD) | 0.008 | 0.141 | 0.171 | 0.401 | –0.425 | 0.911 |
MSE, MAE, and SD are, respectively, the mean signed error, mean absolute error, and standard deviation with respect to experimental values and are given in eV. Max(+) and Max(−) are the largest positive and negative deviations (eV). R2 is the determination coefficient obtained by comparing experimental and theoretical data. Note that the MSE are computed as theory-experiment. For TD-M06-2X, only the results obtained with the largest atomic basis set are displayed. The default PCM model is applied except for when noted as SMD.