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. 2015 Apr 23;2(3):034901. doi: 10.1063/1.4918803

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© 2015 Author(s).

2329-7778/2015/2(3)/034901/19

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FIG. 6. — (a) Dependence of the difference spectrum on the 268 nm pulse energy. The inset shows the absorption peak intensity as a function of UV pulse energy. (b) Comparison of the observed difference spectrum and simulated spectra assuming various K-edge shifts (ΔE) and fractional populations of the photoproducts (f). The simulated spectra are in reasonable agreement with the observed one when ΔE is assumed to be −4 and −5 eV. (c) Reconstructed spectrum of the photoproduct (red) generated from the static spectrum of [Fe(III)(C₂O₄)₃]³⁻ (s = 5/2) (black) and the difference spectrum measured at t = 7 ps (blue), assuming f = 0.5.