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. 2016 Jun 10;7:11873. doi: 10.1038/ncomms11873

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(a) Previous work on C–H activation utilizing substrate control of regioselectivity. (b) Catalytic cycle of halogenase biocatalysis using a Fl-Hal, along with flavin reductase (Fre) and glucose dehydrogenase (GDH) enzymes for cofactor recycling. (c) Proposed scheme of regioselective C–H activation using catalyst control by integration of a Fl-Hal and palladium-catalysed SMC. Biocat., biocatalysis; chemocat., chemocatalysis.