Table 3.
Enzyme | Parameter | PEN | AMP | AMX | TIC | PIP | CER | CEF | CAZ | CTX | FEP | ATM | CLA | SUL | TZB |
---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|---|
SHV-1** | Kcat | 455 | 900 | 60 | 570 | 170 | 10 | NH | NH | >100 | NH | ||||
Km | 20 | 90 | 22 | 60 | 110 | 26 | ND | ND | >3000 | ND | |||||
Kcat/Km | 23,000 | 10,000 | 2700 | 10,000 | 1500 | 400 | ND | ND | >35 | ND | |||||
Vmax/Km | 100 | 4 | 1 | ||||||||||||
Ki | 0.19 | 1.70 | 0.057 | ||||||||||||
IC50 | 0.057 | 7.50 | 0.150 | ||||||||||||
SHV-2 | Ki | 0.16 | 0.36 | 0.04 | |||||||||||
IC50 | 0.020 | 0.57 | 0.049 | ||||||||||||
Vmax | 100 | 6.5 | 70 | 1 | |||||||||||
Km | 3.5 | 12 | ND | ND | 24 | 18 | NA | 10 | |||||||
Kcat | 206 | ND | ND | 11 | NA | ||||||||||
Kcat/Km | 17 | ND | ND | 0.6 | 0.008 | ||||||||||
SHV-2a | Ki | 13 | 5 | 72 | 4 | 3 | 0.08 | 0.47 | 0.027 | ||||||
IC50 | 100 | 53 | 1 | 10 | 0.018 | 0.68 | 0.038 | ||||||||
SHV-4 | Vmax | 100 | 52 | 115 | 5 | ||||||||||
Km | 3.5 | 60 | 25 | 0.5 | |||||||||||
SHV-5 | Ki | 0.10 | 0.18 | 0.036 | |||||||||||
IC50 | 0.005 | 0.40 | 0.022 | ||||||||||||
Km | 15 | 11 | 3 | 23 | 7 | 0.02 | |||||||||
Vmax/Km | 100 | 100 | 51 | 4 | 7 | ||||||||||
SHV-7 | Km | 2.7 | 24 | 11 | 13 | ||||||||||
Vmax | 35 | 13 | 30 | 3.3 | |||||||||||
SHV-9 | Vmax | 100 | 215 | 58 | 10 | 24 | |||||||||
Km | 18 | 12 | 5 | 18 | 9 | ||||||||||
IC50 | 0.14 | 0.43 | |||||||||||||
SHV-13 | Km | 10 | 28 | 18 | 91 | 11 | 77 | ||||||||
Vmax | 100 | 178 | 136 | 0.38 | 12 | 0.66 | |||||||||
Vmax/Km | 100 | 64 | 76 | 0.42 | 11 | 0.86 | |||||||||
SHV-18 | Vmax | 100 | 200 | 13.5 | 26.9 | < 1 | |||||||||
Vmax/Km | 100 | 53 | 1.5 | 24 | ND | ||||||||||
SHV-24 | Vmax | 2 | 2.37 | 0.043 | 0.735 | ||||||||||
Km | 32 | 210 | 30 | 500 | |||||||||||
Vmax/Km | 0.0625 | 0.0113 | 0.000143 | 0.00147 | |||||||||||
Ki | 57 | ND | 37 | ND | |||||||||||
SHV-38$ | Kcat | 100 | 1800 | 10 | 100 | 40 | 5 | 110 | 1 | 3 | 3 | ||||
Km | 13 | 35 | 14 | 80 | 150 | 100 | 3800 | 800 | 1600 | 5500 | |||||
Kcat/Km | 7700 | 51,000 | 700 | 1300 | 270 | 50 | 30 | 1 | 2 | 0.5 | |||||
SHV-55* | Km | 5 ± 0.51 | 10 ± 0.14 | 6 ± 0.02 | 8 ± 0.37 | 9 ± 0.68 | 58 ± 7.40 | 21 ± 0.13 | 149 ± 2.61 | 5 ± 0.62 | |||||
Kcat | 23 ± 0.76 | 23 ± 0.17 | 8 ± 0.00 | 27 ± 1.53 | 38 ± 3.94 | 9 ± 0.21 | 24 ± 0.34 | 30 ± 3.10 | < 0.1 | ||||||
Kcat/Km | 5.3 ± 0.42 | 2.5 ± 0.002 | 1.5 ± 0.00 | 3.7 ± 0.03 | 4.4 ± 0.78 | 0.2 ± 0.02 | 1.1 ± 0.01 | 0.2 ± 0.02 | ND | ||||||
IC50 | 0.02 | ||||||||||||||
SHV-57 | Km | 67 | 30.9 | ||||||||||||
Kcat | 3.8 × 10−3 | 8.6 × 10−4 | |||||||||||||
Kcat/Km | 5.67 × 10−5 | 2.78 × 10−5 | |||||||||||||
Ki | 27 × 103 | 1.16 × 103 | |||||||||||||
SHV-99* | Km | 12 ± 0.11 | 11 ± 0.26 | 5 ± 0.93 | 13 ± 1.43 | 102 ± 11.38 | 136 ± 4.09 | 183 ± 0.72 | 196 ± 0.60 | ||||||
Kcat | 778 ± 616 | 563 ± 8 | 58 ± 2 | 563 ± 13 | 37 ± 2 | < 0.1 | < 0.1 | 0.5 ± 0.001 | |||||||
Kcat/Km | 62.3 ± 4.4 | 49.6 ± 1.8 | 13 ± 2.4 | 43.5 ± 6.5 | 0.37 ± 0.04 | < 0.001 | < 0.001 | 0.003 | |||||||
IC50 | 0.02 | 0.03 | |||||||||||||
SHV-104 | Kcat | 55 | 80 | 30 | >1.8 | ||||||||||
Km | 94 | 10 | 68 | >600 | |||||||||||
Kcat/Km | 0.6 | 8 | 0.44 | 0.003 | |||||||||||
SHV-129#* | Kcat | 22.8 ± 11 | 1688 ± 4 | 26 ± 1 | 3.1 ± 1.5 | 4.8 ± 3.4 | 4.5 ± 0.5 | ||||||||
Km | 46.8 ± 24 | 25 ± 9 | 12.1 ± 3.7 | 24 ± 3 | 26.7 ± 5.5 | 52 ± 3.5 | |||||||||
Kcat/Km | 0.5 ± 0.7 | 7 ± 0.4 | 2.2 ± 0.3 | 0.13 ± 0.5 | 0.2 ± 0.5 | 0.09 ± 0.01 | |||||||||
Ki | 0.4 | 0.4 | 0.04 |
Antibiotic: Penicillin (PEN); Ampicillin (AMP); Amoxicillin (AMX); Ticarcillin (TIC); Piperacillin (PIP); Cephaloridine (CER); Cephalothin (CEF); Ceftazidime (CAZ); Cefotaxime (CTX); Cefepime (FEP); Aztreonam (ATM); Clavulanic Acid (CLA); Sulbactam (SUL); Tazobactam (TZB).
Parameters are expressed as μM (Ki, IC50, Km), s−1(Kcat), and μM/min (Kcat/Km, Vmax). Only antibiotics for which 3 or more SHV enzyme values were available are reported.
NA, not able to determine the rate of hydrolysis and affinity; NH, not hydrolyzed; ND, not determined.
Non ESBL SHV-1 is provided as reference.
Kcat/Km values are expressed as mM/s.
Kcat/Km values are expressed as μM/s.
Values (Except IC50) represent mean ± standard deviation.
References: SHV-1 (Gutmann et al., 1989; Poirel et al., 2003); SHV-2 (Gutmann et al., 1989; Bradford et al., 1995; Winkler and Bonomo, 2016); SHV-2a (Podbielski et al., 1991); SHV-4 (Péduzzi et al., 1989); SHV-5 (Gutmann et al., 1989); SHV-7 (Bradford et al., 1995); SHV-9 (Prinarakis et al., 1996); SHV-13 (Yuan et al., 2000); SHV-18 (Rasheed et al., 2000); SHV-24 (Kurokawa et al., 2000); SHV-38 (Poirel et al., 2003); SHV-55 (Mendonça et al., 2006); SHV-57 (Ma et al., 2005): SHV-99 (Ramdani-Bouguessa et al., 2011); SHV-104 (Ben Achour et al., 2014); SHV-129 (Winkler and Bonomo, 2016).