Figure 3. Metallaphotoredox-catalyzed amination: amine and arene scope.
For each entry number (in boldface), data are reported as percent isolated yield. R, H, alkyl, or aryl substrate; Y, C, CH, or N; X, CI or Br; DABCO, 1,4-diazabicyclo[2.2.2]octane; MTBD, 7-methyl-1,5,7-triazabicyclo [4.4.0]dec-5-ene; LED, light-emitting diode; Me, methyl; n-pent, n-pentyl; Boc, tert-butoxycarbonyl. *Run at ambient temperature. †Reaction heated to 55 °C. ‡DMSO used as solvent. §MTBD used as base. ‖0.002 mol% 1 used. ¶10 mol% pyrrolidine included. #See Supplementary Materials for details.