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. 2016 Oct 24;6:35538. doi: 10.1038/srep35538

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Copyright © 2016, The Author(s)

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PL changes from donors titrated with a mixture of “N” equivalents of AuNCs. (a,d) PL changes of (AuNC)_N/Ru(bpy) system and (AuNC)_N/Tb(chelate), respectively, excited at 470 nm. Inset is the net PL spectral changes from AuNCs representing the sensitized acceptor intensity component. (b,e) Excited state lifetime measurements of Ru(bpy) and Tb(chelate) in (AuNC)_N/donor systems, respectively. Inset plots the conjugation ratio (N) dependence of the donor’s averaged lifetimes. In e, the apparent rise-time differences are attributed to the slow CS-124 to Tb to AuNC transfer processes and are not considered for excited state lifetime calculation. (c,f) Excited state lifetime measurements of AuNC in (AuNC)_N/donor systems. Inset shows the conjugation ratio (N) dependence of the AuNC averaged lifetimes.