(a) Normalized absorption
(green) and photoluminescence (PL) (orange)
spectra of R6G; (b) ASE spectra of the reference R6G solution without
nanostars, excited by single pulses at different excitation fluences
from 0.33 to 0.66 mJ cm–2 in steps of 0.03 mJ cm–2. The intensity of the PL spectra of R6G at a pumping
fluence of 0.24 mJ cm–2 (dashed orange curve) was
magnified 30 times for comparison. (c,e,g,i) Spectral overlap of the
R6G absorption and emission spectra (dotted curves) with the extinction
spectra of respective nanostars in ethanol (solid lines) and (d,f,h,j)
the emission (random lasing or ASE) spectra at different excitations
fluences for nanostars/R6G mixtures. (c,d) AuNSts, (e,f) AuNSts@SiO2, (g,h) AuAgNSts, and (i,j) AuAgNSts@SiO2, respectively.