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. 2016 Dec 20;7:13872. doi: 10.1038/ncomms13872

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Copyright © 2016, The Author(s)

This work is licensed under a Creative Commons Attribution 4.0 International License. The images or other third party material in this article are included in the article's Creative Commons license, unless indicated otherwise in the credit line; if the material is not included under the Creative Commons license, users will need to obtain permission from the license holder to reproduce the material. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/

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(a) The Cu₂(AzoBPDC)₂(AzoBiPyB) membrane, which is initially in the trans state, is irradiated with ultraviolet-light for time intervals of 100 and 200 s, resulting in an increase of the H₂:CO₂ selectivity. (b) The membrane is initially in the cis state and is irradiated with 455 nm for time intervals of 30 and 50 s. (c) Correlation of the H₂:CO₂ separation factor with the ratio of cis azobenzene. The grey triangle and black spheres represent the data from figure (a,b), respectively; the correlation to the cis azobenzene ratio results from the comparison with the IRRAS data, see Supplementary Fig. 6.