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. 2016 May 9;7(8):5236–5248. doi: 10.1039/c6sc00512h

Table 1. Mn EXAFS curve fitting parameters for the HS and LS S2 species a .

Sample Fit # Shell N R σ 2 R/%
LS S2 1 Mn–O 4 1.83 (0.01) 0.005 (0.001) 4.2
Mn–O(N) 2 2.00 (0.03) 0.004 (0.001)
Mn–Mn 1.5 2.72 (0.02) 0.002 (0.002)
Mn–Mn 0.5 3.24 (0.11) 0.005 (0.001)
Mn–Ca 0.75 3.36 (0.01) 0.007 (0.001)
Mn–Ca 0.25 3.89 (0.01) 0.005 (0.001)
E 0 (eV) = –9.3
HS S2 1 Mn–O 4 1.85 (0.03) 0.005 (0.001) 2.6
Mn–O(N) 2 2.05 (0.07) 0.006 (0.006)
Mn–Mn 1.5 2.74 (0.03) 0.004 (0.003)
Mn–Mn 0.5 3.30 (0.07) 0.001 (0.001)
Mn–Ca 0.75 3.36 (0.01) 0.007 (0.001)
Mn–Ca 0.25 4.09 (0.01) 0.015 (0.001)
Mn–C 3 4.39 (0.17) 0.002 (0.001)
E 0 (eV) = –8.1
2 Mn–O 4 1.84 (0.03) 0.005 (0.003) 1.2
Mn–O(N) 2 2.02 (0.06) 0.007 (0.008)
Mn–Mn 1 2.72 (0.02) 0.001 (0.001)
Mn–Mn 1 3.30 (0.05) 0.005 (0.001)
Mn–Ca 0.75 3.26 (0.14) 0.007 (0.001)
Mn–Ca 0.25 4.09 (0.01) 0.006 (0.001)
Mn–C 3 4.35 (0.14) 0.004 (0.001)
E 0 (eV) = –11.2

aS02 was set to 0.85. σ2 is the Debye–Waller factor, R (%) shows the goodness of fit. The fit range of all the spectra are k = 2.4–11.3 Å–1 (R = 1–4.2 Å). Note that for Mn–Mn interactions, N = 1.5 implies that there are three similar interactions within the cluster, as the number of interactions is divided by the number of Mn in the cluster (i.e. 3/4 = 1.5) to be normalized it to per Mn. Similarly, Mn–Ca 0.5 means there are two similar Mn–Ca interactions within the cluster (i.e. 2/4 = 0.5).