Fig. S5.

Fraction crystallized vs. the number of laser pulses, N_p, for a 100-ML (initially) ASW film (black line) and a 75-ML CI plus 25-ML (initially) ASW film (red line). For the 75-ML CI plus 25-ML ASW film, the data show the crystallization of the 25-ML ASW portion of the film. For this plot, the crystallization is reported as the fraction crystallized, whereas for the figures discussed in this report it is given as the amount crystallized (in monolayers). For both experiments, T_max = 225 K. By the time that crystallization of the 100-ML ASW film becomes appreciable (dashed vertical line), the film with the CI template has completely crystallized. Note that the initial linear increase in the red curve is not obvious due to the logarithmic scale for the x axis (Fig. 1E and Fig. S3C for similar data plotted on a linear scale).