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(A) In the wt-β2/α2/CDP/ATP complex, PT from Fe1–H2O to Y122• occurs concomitant with ET from Y356 to Y122•. (B) In the NO2Y122•-β2/α2/CDP/ATP complex, ET from Y356 to Y122• generates the NO2Y– phenolate. RT initiation in F3Y122•-β2 is proposed to generate the F3Y122– phenolate (Scheme 1).
