Table 6.
Entry | R1 | Alkene | Product | Yield [%] | trans/cis |
---|---|---|---|---|---|
1 | Ph | 94 | 78:22 | ||
2 | CN | 68 | 70:30 | ||
3 | NO2 | 63 | 72:28 | ||
4 | OMe | 94 | 74:26 | ||
5 | iPr | 97 | 75:25 | ||
6 | iPr | 93 | 73:26 | ||
7 | iPr | 96 | 75:25 | ||
8 | iPr | 77 | 62:38 | ||
9 | iPr | 89 | 89:11 | ||
10 | iPr | 90 | 86:14 | ||
11 | iPr | 85 | 90:10 |
[a] Reactions were performed under N2 with 1.0 equiv. of sodium tosylhydrazone, 3.0 equiv. alkene, 0.15 equiv. Aliquat®336 and 3 mol % [Co(MeTAA)]. Concentration: 0.675 mmol sodium tosylhydrazone/5 mL THF solvent.