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. 2017 Jul 18;8:77. doi: 10.1038/s41467-017-00041-5

Table 3.

Changes to 24-h mean particle concentrations associated with variation in the gasoline‐ethanol fuel mix

Column number: (1) (2) (3) (4) (5) (6) (7) (8) (9) (10)
Dependent variable: Nucleation Aitken Accumulation BC PM2.5
Unit: dN/dlogDp, cm−3 dN/dlogDp, cm−3 dN/dlogDp, cm−3 µg m−3 µg m−3
Mean over hour window: 24-h 24-h 24-h 24-h 24-h
Sample period: Oct/2010 to Oct/2010 to Oct/2010 to Oct/2010 to Nov/2008 to
May/2011 May/2011 May/2011 Apr/2011 and Oct to Nov/2012 May/2013
Number of sampling sites: 1 1 1 1 3
Source: Own Own Own Own CETESB
Estimation: 2-step model 2SLS model 2-step model 2SLS model 2-step model 2SLS model 2-step model 2SLS model 2-step model 2SLS model
Flex fuel share of Gasoline E20/E25 rises from 30 to 80% 2,794 ± 1,456 2,783 ± 1,433 332 ± 818 361 ± 818 565 ± 785 553 ± 806 1.1 ± 1.3 1.0 ± 1.2 0.2 ± 3.9 −0.2 ± 2.9
Equivalently, share of Ethanol E100 falls from 70 to 20%
Control variables (to correct for the influence of other determinants of particles)
Site-specific linear trend Yes Yes Yes Yes Yes Yes Yes Yes Yes Yes
Quarter-of-year fixed effects Yes Yes Yes Yes Yes Yes Yes Yes
Week-of-year fixed effects Yes Yes
Day-of-week fixed effects Yes Yes Yes Yes Yes Yes Yes Yes Yes Yes
Radiation (+100 W m−2) −234 ± 664 −235 ± 607 110 ± 386 111 ± 361 108 ± 259 108 ± 226 0.0 ± 0.3 0.0 ± 0.2 −0.4 ± 2.2 −0.3 ± 1.3
Temperature (+1 oC) −499 ± 234 −498 ± 211 −61 ± 119 −63 ± 105 32 ± 100 32 ± 91 0.1 ± 0.1 0.1 ± 0.1 1.2 ± 0.5 1.2 ± 0.4
Humidity (+10%) −1,454 ± 699 −1,453 ± 543 −715 ± 384 −718 ± 322 −97 ± 265 −96 ± 243 −0.4 ± 0.2 −0.4 ± 0.2 −1.0 ± 1.6 −1.0 ± 1.2
Wind speed (+1 m s−1) −569 ± 1,144 −567 ± 1,046 −1,910 ± 686 −1,913 ± 593 −485 ± 449 −484 ± 389 −1.6 ± 0.6 −1.6 ± 0.5 −6.5 ± 2.8 −6.5 ± 2
Other meteorolog. and road traffic conditions (see notes) Yes Yes Yes Yes Yes Yes Yes Yes Yes Yes
R 2 57.3% 57.3% 51.5% 51.5% 54.5% 54.5% 74.1% 74.1% 73.4% 73.4%
Number of observations 198 198 198 198 198 198 228 228 511 511
Number of regressors 30 30 30 30 30 30 29 29 74 74
Mean value of dependent variable 8,755 8,755 3,320 3,320 1,494 1,494 3.3 3.3 13.8 13.8

Coefficients and 95% confidence intervals, i.e., point estimate ± 2 standard errors. An observation is a date (columns 1–8) or a date-site pair (columns 9–10). Samples exclude the colder months of June to September and include all days of the week. Radiation, temperature, humidity, and wind speed in the recorded unit. All columns additionally include several wind direction, precipitation, thermal inversion and road traffic congestion indicators. Since the longer sample encompasses 2010, columns 9–10 include site-specific intercepts indicating the opening of the Greater São Paulo beltway’s southern section on March 31, 2010. The effect of raising the gasoline share in the flex fleet is scaled for in-sample variation from 30 to 80%. The corresponding variation in the ethanol share is one minus variation in the gasoline share. Ordinary Least Squares estimates in the odd-numbered columns, with standard errors calculated by bootstrapping (200 samples each): (i) the consumer-level fuel choice data, to account for sampling variation in the predicted gasoline share in a first-step consumer demand model, and (ii) the pollutant-meterology-traffic data in the second-step particle regression, clustering by date. Two-Stage Least Squares estimates in the even-numbered columns, with the median ethanol-to-gasoline price ratio across pumping stations instrumenting for the predicted gasoline share in the particle regression equation